Magnetic remote actuation of soft materials is attractive for applications such as transforming materials and medical robots. However, due to manufacturing limitations, microscale magnetoactive devices are scarce and light-based additive manufacturing methods, despite achieving microscale resolution, struggle with particle-induced light scattering. Moreover, large hard-magnetic microparticles restrict ultimate feature sizes and deformation of soft-magnetic nanoparticle composites […]
We present a modular design strategy for the one-step fabrication of arrays of magnetically responsive microactuators connected to the substrate via compliant hinges. We use direct laser writing in the form of two-photon crosslinking within bilayer films to generate three-dimensional microstructures in which magnetic nanoparticles are embedded in the upper layer. This part of the […]
Mechanical forces play a crucial role in many biological processes, including cell–cell and cell–matrix interactions. The generation of surface-attached multilayer micromagnet systems fabricated by two-photon lithography and the use of such systems to perform single-cell actuation are presented. The actuators are generated by two-photon crosslinking and consist of a soft and flexible surface-attached hydrogel layer […]
Direct laser writing has gained remarkable popularity by offering architectural control of 3D objects at submicron scales. However, it faces limitations when the fabrication of microstructures comprising multiple materials is desired. The generation processes of multi-material microstructures are often very complex, requiring meticulous alignment, as well as a series of step-and-repeat writing and development of […]
Surface-bound 3D micro-magnets are fabricated from photoreactive copolymers filled with magnetic nanoparticles by maskless 3D writing. The structures are generated by 2-photon crosslinking (2PC), which allows direct writing into solid films of composites consisting of magnetic particles and a photoreactive elastomer precursor. With this strategy, it is possible to directly write complex, surface-bound magnetic actuator […]
Acrylate-endcapped urethane-based precursors constituting a poly(D,L-lactide)/poly(ε-caprolactone) (PDLLA/PCL) random copolymer backbone are synthesized with linear and star-shaped architectures and various molar masses. It is shown that the glass transition and thus the actuation temperature could be tuned by varying the monomer content (0–8 wt% ε-caprolactone, Tg,crosslinked = 10—42 °C) in the polymers. The resulting polymers are […]
